Halogen compounds are important intermediates in organic synthesis and have many industrial applications.
Overview
graph TD
A[Halogen Compounds] --> B[Haloalkanes]
A --> C[Haloarenes]
B --> B1[Preparation]
B --> B2[Reactions]
C --> C1[Properties]
C --> C2[Reactions]Classification
By Halogen Position
- Primary: Halogen on primary carbon
- Secondary: Halogen on secondary carbon
- Tertiary: Halogen on tertiary carbon
Nature of C-X Bond
- Polar covalent
- Carbon is electrophilic
- Bond strength: C-F > C-Cl > C-Br > C-I
- Reactivity: C-I > C-Br > C-Cl > C-F
Preparation of Haloalkanes
From Alcohols
$$\text{R-OH} + \text{HX} \rightarrow \text{R-X} + \text{H}_2\text{O}$$Reactivity: 3° > 2° > 1°
Other reagents: PCl₃, PCl₅, SOCl₂
Halogenation of Alkanes
$$\text{R-H} + \text{X}_2 \xrightarrow{h\nu} \text{R-X} + \text{HX}$$Free radical mechanism
From Alkenes
Addition of HX:
$$\text{R-CH=CH}_2 + \text{HX} \rightarrow \text{R-CHX-CH}_3$$Follows Markovnikov’s rule
Reactions of Haloalkanes
Nucleophilic Substitution
$$\text{R-X} + \text{Nu}^- \rightarrow \text{R-Nu} + \text{X}^-$$SN1 Mechanism:
- Two steps: ionization then attack
- Favored by: 3° substrate, polar protic solvent
- Racemization occurs
SN2 Mechanism:
- One step: backside attack
- Favored by: 1° substrate, polar aprotic solvent
- Walden inversion (stereochemistry inverted)
Elimination (E1 and E2)
Forms alkenes by removing HX.
Saytzeff’s Rule: More substituted alkene is major product.
Haloarenes
Preparation
Sandmeyer Reaction:
$$\text{ArN}_2^+ + \text{CuX} \rightarrow \text{ArX}$$Properties
- Less reactive than haloalkanes
- Due to resonance with benzene ring
- C-X bond has partial double bond character
Reactions
Nucleophilic Substitution: Difficult (activated by -NO₂ groups)
Electrophilic Substitution: ortho/para directing but deactivating
Polyhalogen Compounds
Chloroform (CHCl₃)
- Anesthetic (historically)
- Oxidizes to phosgene (toxic)
Carbon Tetrachloride (CCl₄)
- Fire extinguisher (not used now)
- Dry cleaning solvent
Freons
- CFCs like CCl₂F₂
- Ozone depletion
- Replaced by HFCs
DDT
- Insecticide
- Persistent organic pollutant
- Banned in many countries
Practice Problems
Arrange in order of SN2 reactivity: 1-bromobutane, 2-bromobutane, 2-bromo-2-methylpropane
Explain why chlorobenzene is less reactive than chloroethane in nucleophilic substitution.
What product is obtained when 2-bromopentane reacts with alcoholic KOH?
Further Reading
- Hydrocarbons - Parent hydrocarbons
- Oxygen Compounds - Alcohols and ethers