Benzene and Aromatic Compounds

Master benzene structure, aromaticity criteria, resonance, and electrophilic aromatic substitution mechanisms for JEE

The Hook: The Mystery Molecule That Defied Logic

Connect: Real Life → Chemistry

In 1825, Michael Faraday discovered a mysterious compound in illuminating gas - molecular formula C₆H₆. Scientists were puzzled: such a high degree of unsaturation should make it extremely reactive, yet this compound was remarkably stable!

Even more mysterious: It didn’t behave like alkenes at all!

  • Didn’t decolorize Br₂ readily
  • Didn’t give addition reactions easily
  • Preferred substitution over addition

The JEE question: How can a molecule with four degrees of unsaturation (equivalent to four π bonds!) be so stable? The answer revolutionized organic chemistry: Aromaticity!

Fun fact: Benzene is the smell in petrol/gasoline, and it’s found in coal tar, crude oil, and even coffee!


The Core Concept

What is Benzene?

Benzene (C₆H₆) is the parent aromatic hydrocarbon with a unique cyclic structure that exhibits exceptional stability.

Molecular Formula: C₆H₆

Structure: Hexagonal planar ring with delocalized π electrons

        H
        |
    H—C   C—H
      ║   ║
    H—C   C—H
        |
        H

But this structure doesn’t tell the full story!

The Puzzle of Benzene Structure

Degree of Unsaturation:

$$\text{DBE} = \frac{2C + 2 - H}{2} = \frac{2(6) + 2 - 6}{2} = 4$$

Four degrees of unsaturation suggest:

  • Four double bonds OR
  • Three double bonds + one ring OR
  • Two double bonds + two rings OR
  • One triple bond + one double bond, etc.
Kekulé's Structure (1865)

August Kekulé proposed alternating single and double bonds in a hexagon:

    C═C
   ╱   ╲
  C     C
  ║     ║
  C     C
   ╲   ╱
    C═C

Problems with this structure:

  1. Should have different C-C bond lengths

    • C=C: 134 pm (double bond)
    • C-C: 154 pm (single bond)
    • Reality: All C-C bonds are 139 pm (intermediate!)
  2. Should give two isomers of 1,2-dibromobenzene

    • One with Br on C=C (short distance)
    • One with Br on C-C (long distance)
    • Reality: Only one isomer exists!
  3. Should readily undergo addition (like alkenes)

    • Reality: Prefers substitution!

Conclusion: Simple alternating structure is inadequate!

Modern Picture: Resonance and Delocalization

Resonance Structures:

Benzene is represented as a resonance hybrid of two Kekulé structures:

    C═C              C—C
   ╱   ╲            ╱   ╲
  C     C    ↔    C     C
  ║     ║          ║     ║
  C     C          C     C
   ╲   ╱            ╲   ╱
    C═C              C═C

Better representation: Circle inside hexagon (showing delocalized π electrons)

Reality:

  • All six C-C bonds are equivalent
  • Each C-C bond is partial double bond (bond order = 1.5)
  • Bond length: 139 pm (between 134 and 154 pm)
  • Six π electrons delocalized over entire ring
Resonance Energy

Resonance Energy = Extra stability due to delocalization

For benzene: 152 kJ/mol

What this means:

  • Benzene is 152 kJ/mol more stable than hypothetical cyclohexatriene
  • This extra stability explains why benzene resists addition reactions
  • Adding across double bond would destroy aromaticity (lose 152 kJ/mol of stability!)

JEE Concept: This is why benzene undergoes substitution (retains aromaticity) rather than addition (loses aromaticity)

Related: Chemical Bonding

Interactive Demo: Visualize Benzene’s Aromatic Structure

Explore the delocalized π-electron system that makes benzene so stable.


Aromaticity: Hückel’s Rule

Criteria for Aromaticity

For a compound to be aromatic, it must satisfy ALL four conditions:

The Four Rules of Aromaticity

1. Cyclic Structure

  • Compound must have a closed ring of atoms

2. Planar Structure

  • All atoms in the ring must lie in the same plane
  • Required for π orbital overlap

3. Complete Conjugation (Continuous π System)

  • Every atom in the ring must have a p-orbital
  • Usually means sp² or sp hybridized carbons
  • p-orbitals overlap to form continuous π system

4. Hückel’s Rule: (4n + 2) π electrons

$$\boxed{\text{Number of } \pi \text{ electrons} = 4n + 2, \text{ where } n = 0, 1, 2, 3...}$$

Allowed values: 2, 6, 10, 14, 18… π electrons

Aromatic: 6 π electrons is most common (n=1)

Benzene Satisfies All Criteria

  1. Cyclic: Six-membered ring
  2. Planar: All carbons sp² hybridized, hexagon is flat
  3. Conjugated: Each carbon has one p-orbital, continuous overlap
  4. Hückel’s Rule: 6 π electrons (4×1 + 2 = 6, where n=1)

Conclusion: Benzene is aromatic!

Examples: Aromatic vs Non-Aromatic vs Anti-Aromatic

Classification Guide

AROMATIC (Extra stable, 4n+2 π electrons)

  • Benzene (C₆H₆): 6 π electrons ✓
  • Naphthalene (C₁₀H₈): 10 π electrons ✓
  • Pyridine (C₅H₅N): 6 π electrons ✓
  • Furan (C₄H₄O): 6 π electrons ✓

ANTI-AROMATIC (Highly unstable, 4n π electrons)

  • Cyclobutadiene: 4 π electrons ✗
  • Cyclooctatetraene (if planar): 8 π electrons ✗

Note: Cyclooctatetraene is actually non-planar (tub-shaped) to avoid anti-aromaticity!

NON-AROMATIC (Normal stability, doesn’t follow rules)

  • Cyclohexene: Not fully conjugated ✗
  • Cyclooctatetraene: Not planar ✗
  • Cyclohexane: No π electrons ✗

JEE Tip: If 4n π electrons and planar → Anti-aromatic (very unstable)

Memory Trick: Hückel's Rule

“Hückel’s Magic Numbers: 2, 6, 10, 14…”

For quick checking:

  • n=0: 2 π electrons (rare, but possible)
  • n=1: 6 π electrons ← Most common (benzene!)
  • n=2: 10 π electrons (naphthalene)
  • n=3: 14 π electrons (anthracene)

Anti-aromatic numbers to AVOID: 4, 8, 12, 16… (4n with n=1,2,3…)

JEE Shortcut: Count π electrons

  • If 6 or 10 → Likely aromatic (if planar and cyclic)
  • If 4 or 8 → Anti-aromatic (highly unstable)

Reactions of Benzene: Electrophilic Aromatic Substitution

Key Point: Benzene undergoes substitution (not addition) to preserve aromaticity!

General Mechanism:

$$\boxed{\text{C}_6\text{H}_6 + \text{E}^+ \xrightarrow{\text{catalyst}} \text{C}_6\text{H}_5\text{-E} + \text{H}^+}$$

General Mechanism (Two Steps)

Step 1: Electrophilic Attack → Carbocation Intermediate

    Benzene  +  E⁺
   Arenium ion (σ complex/Wheland intermediate)

      H  E
       \/
      /  \
  • Electrophile attacks π electrons
  • Carbocation intermediate forms (loses aromaticity temporarily!)
  • This is the slow, rate-determining step

Step 2: Deprotonation → Restoration of Aromaticity

   Arenium ion  →  C₆H₅-E  +  H⁺
  • Lose H⁺ to restore aromaticity
  • Fast step
  • Aromaticity regained!

Why substitution, not addition?

$$\Delta G_{\text{sub}} < \Delta G_{\text{add}}$$
  • Substitution: Regains aromatic stability (−152 kJ/mol)
  • Addition: Loses aromatic stability permanently
Key Insight

Benzene “prefers to stay aromatic”

Even though the carbocation intermediate is less stable (lost aromaticity), the system immediately eliminates H⁺ to restore the aromatic ring.

This is the defining characteristic of aromatic compounds!


Specific Reactions of Benzene

Reaction 1: Halogenation

Chlorination

$$\boxed{\text{C}_6\text{H}_6 + \text{Cl}_2 \xrightarrow{\text{FeCl}_3} \text{C}_6\text{H}_5\text{Cl} + \text{HCl}}$$

Mechanism:

Step 1: Generation of electrophile (Cl⁺)

$$\text{Cl}_2 + \text{FeCl}_3 \rightarrow \text{Cl}^+ + [\text{FeCl}_4]^-$$

FeCl₃ is a Lewis acid (electron pair acceptor) - polarizes Cl₂

Step 2: Electrophilic attack

$$\text{C}_6\text{H}_6 + \text{Cl}^+ \rightarrow \text{C}_6\text{H}_6\text{Cl}^+ \text{ (arenium ion)}$$

Step 3: Deprotonation

$$\text{C}_6\text{H}_6\text{Cl}^+ \rightarrow \text{C}_6\text{H}_5\text{Cl} + \text{H}^+$$

Bromination: Similar mechanism with Br₂/FeBr₃ or Br₂/AlBr₃

JEE Trap: Why Need Catalyst?

Q: Why doesn’t benzene react with Cl₂ directly (without FeCl₃)?

Wrong answer: “Benzene is unreactive”

Correct answer:

  • Cl₂ is not electrophilic enough to attack benzene’s π electrons
  • FeCl₃ polarizes Cl-Cl bond: Cl-Cl → Cl^(δ+)-Cl^(δ-)
  • Generates Cl⁺ (strong electrophile)
  • Without catalyst, no reaction at room temperature

Contrast with alkenes:

  • Alkenes have exposed π electrons (above/below plane)
  • React with Cl₂ directly without catalyst
  • Benzene’s π electrons are delocalized → less reactive

JEE One-liner: “Benzene needs catalyst, alkenes don’t”

Reaction 2: Nitration

Formation of Nitrobenzene

$$\boxed{\text{C}_6\text{H}_6 + \text{HNO}_3 \xrightarrow{\text{conc. H}_2\text{SO}_4} \text{C}_6\text{H}_5\text{NO}_2 + \text{H}_2\text{O}}$$

Mechanism:

Step 1: Generation of nitronium ion (NO₂⁺)

$$\text{HNO}_3 + 2\text{H}_2\text{SO}_4 \rightarrow \text{NO}_2^+ + \text{H}_3\text{O}^+ + 2\text{HSO}_4^-$$

Detailed:

$$\text{HNO}_3 + \text{H}_2\text{SO}_4 \rightarrow \text{H}_2\text{NO}_3^+ + \text{HSO}_4^-$$ $$\text{H}_2\text{NO}_3^+ \rightarrow \text{NO}_2^+ + \text{H}_2\text{O}$$

Step 2: Electrophilic attack by NO₂⁺

$$\text{C}_6\text{H}_6 + \text{NO}_2^+ \rightarrow \text{C}_6\text{H}_6(\text{NO}_2)^+ \text{ (arenium ion)}$$

Step 3: Deprotonation

$$\text{C}_6\text{H}_6(\text{NO}_2)^+ \rightarrow \text{C}_6\text{H}_5\text{NO}_2 + \text{H}^+$$

Product: Nitrobenzene (pale yellow liquid, almond-like odor)

Uses:

  • Reduction → Aniline (important dye intermediate)
  • Precursor for explosives (TNT)

Related: Nitrogen Compounds

Reaction 3: Sulfonation

Formation of Benzenesulfonic Acid

$$\boxed{\text{C}_6\text{H}_6 + \text{H}_2\text{SO}_4 \xrightarrow{\text{fuming H}_2\text{SO}_4} \text{C}_6\text{H}_5\text{SO}_3\text{H} + \text{H}_2\text{O}}$$

Fuming H₂SO₄ = Concentrated H₂SO₄ + SO₃ (oleum)

Mechanism:

Step 1: Electrophile = SO₃ (or HSO₃⁺)

$$\text{SO}_3 \text{ acts as electrophile}$$

Step 2: Electrophilic attack

$$\text{C}_6\text{H}_6 + \text{SO}_3 \rightarrow \text{C}_6\text{H}_6(\text{SO}_3)^+ $$

Step 3: Deprotonation

$$\text{C}_6\text{H}_6(\text{SO}_3)^+ + \text{H}_2\text{O} \rightarrow \text{C}_6\text{H}_5\text{SO}_3\text{H} + \text{H}^+$$

Special property: Sulfonation is reversible!

$$\text{C}_6\text{H}_5\text{SO}_3\text{H} + \text{H}_2\text{O} \xrightarrow{\text{heat, steam}} \text{C}_6\text{H}_6 + \text{H}_2\text{SO}_4$$

Use: Sulfonation followed by desulfonation can be used to block a position temporarily in multi-step synthesis!

Reaction 4: Friedel-Crafts Alkylation

Adding alkyl group (R-)

$$\boxed{\text{C}_6\text{H}_6 + \text{R-Cl} \xrightarrow{\text{AlCl}_3} \text{C}_6\text{H}_5\text{-R} + \text{HCl}}$$

Example:

$$\text{C}_6\text{H}_6 + \text{CH}_3\text{Cl} \xrightarrow{\text{AlCl}_3} \text{C}_6\text{H}_5\text{-CH}_3 + \text{HCl}$$

(Benzene → Toluene)

Mechanism:

Step 1: Generation of carbocation

$$\text{R-Cl} + \text{AlCl}_3 \rightarrow \text{R}^+ + [\text{AlCl}_4]^-$$

Step 2: Electrophilic attack

$$\text{C}_6\text{H}_6 + \text{R}^+ \rightarrow \text{C}_6\text{H}_6\text{R}^+$$

Step 3: Deprotonation

$$\text{C}_6\text{H}_6\text{R}^+ \rightarrow \text{C}_6\text{H}_5\text{R} + \text{H}^+$$
JEE Trap: Carbocation Rearrangement!

Common mistake: Expecting primary carbocation to stay as-is

Example:

$$\text{C}_6\text{H}_6 + \text{CH}_3\text{CH}_2\text{Cl} \xrightarrow{\text{AlCl}_3} ?$$

Expected: C₆H₅-CH₂-CH₃ (ethylbenzene)

Reality: Mixture!

  • Some ethylbenzene
  • Also get C₆H₅-CH(CH₃)₂ (isopropylbenzene)

Why?

$$\text{CH}_3\text{CH}_2^+ \rightarrow \text{CH}_3\text{CH}_2^+ \text{ (1°)} $$

Can rearrange via hydride shift:

$$\text{CH}_3\text{-CH}_2^+ \xrightarrow{\text{H-shift}} \text{CH}_3\text{-CH}^+\text{-H} \text{ (wait, this doesn't work)}$$

Actually for ethyl:

$$\text{CH}_3\text{CH}_2^+ \text{ is primary, stays as-is}$$

Better example: n-propyl chloride

$$\text{CH}_3\text{CH}_2\text{CH}_2\text{Cl} + \text{AlCl}_3 \rightarrow \text{CH}_3\text{CH}_2\text{CH}_2^+ \text{ (1°)}$$

Rearranges to:

$$\text{CH}_3\text{CH}^+\text{CH}_3 \text{ (2°, more stable!)}$$

Product: Mainly isopropylbenzene, not n-propylbenzene!

JEE Rule: “Friedel-Crafts with 1° halides → Expect rearrangements!”

To avoid: Use acyl chlorides (Friedel-Crafts acylation) - no rearrangement!

Limitations of Friedel-Crafts Alkylation:

  1. Polyalkylation - Product is more reactive than starting material
  2. Carbocation rearrangement - Especially with 1° and 2° halides
  3. Doesn’t work with deactivated rings (nitrobenzene, etc.)

Reaction 5: Friedel-Crafts Acylation

Adding acyl group (R-CO-)

$$\boxed{\text{C}_6\text{H}_6 + \text{R-CO-Cl} \xrightarrow{\text{AlCl}_3} \text{C}_6\text{H}_5\text{-CO-R} + \text{HCl}}$$

Example:

$$\text{C}_6\text{H}_6 + \text{CH}_3\text{COCl} \xrightarrow{\text{AlCl}_3} \text{C}_6\text{H}_5\text{-CO-CH}_3$$

(Benzene → Acetophenone)

Mechanism:

Step 1: Generation of acylium ion

$$\text{R-CO-Cl} + \text{AlCl}_3 \rightarrow [\text{R-C≡O}]^+ + [\text{AlCl}_4]^-$$

Acylium ion: R-C≡O⁺ (resonance stabilized, doesn’t rearrange!)

Step 2: Electrophilic attack

$$\text{C}_6\text{H}_6 + [\text{R-C≡O}]^+ \rightarrow \text{C}_6\text{H}_6(\text{COR})^+$$

Step 3: Deprotonation

$$\text{C}_6\text{H}_6(\text{COR})^+ \rightarrow \text{C}_6\text{H}_5\text{-CO-R} + \text{H}^+$$

Advantages over alkylation:

  1. No rearrangement - Acylium ion is resonance stabilized
  2. No polyacylation - Product (ketone) is deactivated, won’t react further
  3. Can reduce to alkyl - Reduce C₆H₅-CO-R → C₆H₅-CH₂-R (Clemmensen/WK)
JEE Strategy: Alkylation vs Acylation

Want to add alkyl group to benzene?

Direct alkylation issues:

  • Polysubstitution
  • Rearrangement (for 1°, 2° carbocations)

Better approach: Acylation followed by reduction!

$$\text{C}_6\text{H}_6 \xrightarrow[\text{AlCl}_3]{\text{RCOCl}} \text{C}_6\text{H}_5\text{-CO-R} \xrightarrow{\text{Zn-Hg/HCl}} \text{C}_6\text{H}_5\text{-CH}_2\text{-R}$$

Benefits:

  • No polysubstitution (ketone deactivates ring)
  • No rearrangement (acylium ion is stable)
  • Clean, single product

JEE Mantra: “For clean alkylation, go via acylation!”

Related: Carbonyl Compounds


Orientation in Disubstituted Benzenes

Quick preview - Detailed coverage in Directive Effects

When benzene already has one substituent, where does the second group attach?

Three positions possible:

       R
       |
    1  2  ortho (o-)
   6      3  meta (m-)
    5  4  para (p-)
  • Ortho (o-): Adjacent to existing group (positions 2, 6)
  • Meta (m-): One carbon away (positions 3, 5)
  • Para (p-): Opposite side (position 4)

Substituents are classified as:

  1. Ortho-para directors (OH, NH₂, CH₃, halogens)

    • Direct incoming group to ortho and para positions
    • Most are activating (make ring more reactive)
    • Exception: Halogens are deactivating but still o/p-directing
  2. Meta directors (NO₂, SO₃H, COOH, CN)

    • Direct incoming group to meta position
    • All are deactivating (make ring less reactive)
Memory Trick

“Electron Donating = Ortho/Para” “Electron Withdrawing = Meta”

Exception: Halogens (withdraw by induction, donate by resonance)

  • Net effect: Deactivating
  • But still ortho/para directors (resonance wins for orientation!)

Detailed mechanisms and examples in next topic: Directive Effects


Common Mistakes to Avoid

Mistake #1: Confusing Aromaticity Rules

Wrong: “Benzene has 3 π bonds, so 3 × 2 = 6 π electrons”

Correct thinking process:

  • Count total π electrons in the system
  • Don’t count π bonds separately
  • Each C contributes 1 p-electron
  • 6 carbons × 1 electron = 6 π electrons total
  • Check if 4n+2 (n=1): 4(1)+2 = 6 ✓

JEE Trap: Some students count double bonds instead of electrons

Mistake #2: Expecting Addition Reactions

Wrong: Benzene + Br₂ → C₆H₆Br₂ (addition product)

Correct: Benzene + Br₂/FeBr₃ → C₆H₅Br (substitution product)

Why?

  • Addition would destroy aromaticity (lose 152 kJ/mol stability!)
  • Substitution preserves aromaticity
  • System “prefers” to regain aromatic stabilization

JEE Rule: Aromatic compounds → Substitution, not addition

Mistake #3: Forgetting Catalyst Requirement

Wrong: Benzene reacts with Cl₂ at room temperature

Correct: Need FeCl₃ or AlCl₃ catalyst to generate Cl⁺

Why benzene needs catalyst but alkenes don’t:

PropertyAlkenesBenzene
π electronsLocalized, exposedDelocalized, stable
ReactivityHighLow (aromatic stability)
ElectrophileCl₂ sufficientNeed Cl⁺ (stronger)

JEE Tip: Always write catalyst in benzene reactions!


Practice Problems

Level 1: Foundation (NCERT)

Problem 1: Structure and Stability

Q: Why does benzene show exceptional stability compared to hypothetical cyclohexatriene?

Solution:

Key concept: Resonance energy

Comparison:

Hypothetical cyclohexatriene:

  • Three localized C=C double bonds
  • Three C-C single bonds
  • Alternating bond lengths

Actual benzene:

  • Six π electrons delocalized over entire ring
  • All C-C bonds equivalent (139 pm)
  • Resonance stabilization = 152 kJ/mol

Answer: Delocalization of π electrons over the entire ring provides extra stability (resonance energy of 152 kJ/mol), making benzene much more stable than expected for a compound with three double bonds.

Practical consequence: Resists addition reactions (would lose aromaticity)

Problem 2: Aromaticity Test

Q: Is cyclooctatetraene (C₈H₈) aromatic?

Solution:

Check all four criteria:

  1. Cyclic? Yes ✓
  2. Planar? NO ✗ (tub-shaped to avoid anti-aromaticity)
  3. Conjugated? Would be if planar
  4. Hückel’s rule? 8 π electrons = 4n (n=2) ✗

Count π electrons: 4 C=C double bonds = 8 π electrons

Check Hückel: 4n+2 = ?

  • If n=1: 4(1)+2 = 6 ✗
  • 8 = 4(2) = 4n → Anti-aromatic if planar!

Reality: To avoid anti-aromaticity, cyclooctatetraene adopts non-planar tub shape

Answer: NOT aromatic (it’s non-aromatic because not planar)

JEE Insight: 8 π electrons would be anti-aromatic if planar, so molecule distorts to avoid this!

Level 2: JEE Main

Problem 3: Mechanism Understanding

Q: Why does benzene undergo electrophilic substitution rather than electrophilic addition?

Solution:

Energy considerations:

Addition pathway:

$$\text{C}_6\text{H}_6 + \text{Br}_2 \rightarrow \text{C}_6\text{H}_6\text{Br}_2$$
  • Loses aromaticity permanently
  • Loses 152 kJ/mol resonance energy
  • Product has no special stability

Substitution pathway:

$$\text{C}_6\text{H}_6 + \text{Br}_2 \xrightarrow{\text{FeBr}_3} \text{C}_6\text{H}_5\text{Br} + \text{HBr}$$
  • Temporarily loses aromaticity (arenium intermediate)
  • Regains aromaticity in product
  • Net: Retains aromatic stabilization

Energy diagram:

Energy
  |    ‡ (Arenium ion)
  |   /\
  |  /  \___  C₆H₅Br + HBr (aromatic - stable)
  | /
  |/___________  C₆H₆ (aromatic - stable)
  |

Answer: Substitution pathway allows benzene to regain its aromatic stability, making it thermodynamically and kinetically more favorable than addition which permanently destroys aromaticity.

JEE Key Point: Loss of 152 kJ/mol is too costly!

Problem 4: Reaction Products

Q: What is the major product when benzene reacts with CH₃CH₂COCl in presence of AlCl₃?

Solution:

This is Friedel-Crafts Acylation

Reagent: CH₃CH₂COCl (propanoyl chloride)

Step 1: Form acylium ion

$$\text{CH}_3\text{CH}_2\text{COCl} + \text{AlCl}_3 \rightarrow [\text{CH}_3\text{CH}_2\text{C≡O}]^+ + [\text{AlCl}_4]^-$$

Step 2: Electrophilic substitution

$$\text{C}_6\text{H}_6 + [\text{CH}_3\text{CH}_2\text{C≡O}]^+ \rightarrow \text{C}_6\text{H}_5\text{-CO-CH}_2\text{CH}_3 + \text{H}^+$$

Product: Propiophenone (C₆H₅-CO-CH₂-CH₃)

Key points:

  • No rearrangement (acylium ion is stable)
  • Only monosubstitution (product is deactivated)
  • Clean, predictable reaction

Answer: C₆H₅-CO-CH₂-CH₃ (propiophenone)

Level 3: JEE Advanced

Problem 5: Aromaticity Analysis

Q: Arrange the following in order of increasing aromatic character: (a) Benzene (b) Cyclopentadienyl anion (C₅H₅⁻) (c) Cycloheptatrienyl cation (C₇H₇⁺, tropylium) (d) Pyrrole (C₄H₄NH)

Solution:

Check each for aromaticity:

(a) Benzene (C₆H₆):

  • 6 π electrons (4×1+2) ✓
  • Planar ✓
  • Cyclic, conjugated ✓
  • Aromatic

(b) Cyclopentadienyl anion (C₅H₅⁻):

    [  ]⁻
  • 5 carbons, each contributes 1 π electron = 5
  • Plus negative charge (2 electrons in p-orbital) = 6 total
  • 6 π electrons (4×1+2) ✓
  • Planar ✓
  • Aromatic (remarkably stable for anion!)

(c) Tropylium cation (C₇H₇⁺):

    [  ]⁺
  • 7 carbons, but one has empty p-orbital (positive charge)
  • 3 double bonds = 6 π electrons
  • 6 π electrons ✓
  • Planar ✓
  • Aromatic (remarkably stable for cation!)

(d) Pyrrole (C₄H₄NH):

    NH
    ||
   /  \
  • 4 carbons: 2 double bonds = 4 π electrons
  • N has lone pair in p-orbital = 2 π electrons
  • Total: 4 + 2 = 6 π electrons ✓
  • Planar ✓
  • Aromatic

All are aromatic! But question asks for “increasing aromatic character”

Consider resonance energy and stability:

Resonance energies (approximate):

  • Benzene: 152 kJ/mol (most stable, perfect symmetry)
  • Tropylium: ~150 kJ/mol
  • Cyclopentadienyl: ~105 kJ/mol
  • Pyrrole: ~90 kJ/mol (heteroatom disrupts symmetry)

Order: Pyrrole < Cyclopentadienyl anion < Tropylium < Benzene

Answer: (d) < (b) < (c) < (a)

JEE Insight:

  • All satisfy Hückel’s rule (6 π electrons)
  • But resonance energy varies
  • Benzene is “gold standard” for aromaticity
  • Ions and heteroaromatic compounds have lower resonance energy

Related: Heterocyclic Compounds

Problem 6: Multi-Step Synthesis

Q: How will you convert benzene to n-propylbenzene using Friedel-Crafts reaction?

Solution:

Target: C₆H₅-CH₂-CH₂-CH₃

Problem: Direct alkylation with n-propyl chloride gives rearrangement!

$$\text{C}_6\text{H}_6 + \text{CH}_3\text{CH}_2\text{CH}_2\text{Cl} \xrightarrow{\text{AlCl}_3} \text{C}_6\text{H}_5\text{CH(CH}_3\text{)}_2$$

(isopropylbenzene, major)

Why? 1° carbocation rearranges to 2°:

$$\text{CH}_3\text{-CH}_2\text{-CH}_2^+ \rightarrow \text{CH}_3\text{-CH}^+\text{-CH}_3$$

Solution: Use Friedel-Crafts Acylation + Reduction

Step 1: Acylation (no rearrangement!)

$$\text{C}_6\text{H}_6 + \text{CH}_3\text{CH}_2\text{COCl} \xrightarrow{\text{AlCl}_3} \text{C}_6\text{H}_5\text{-CO-CH}_2\text{CH}_3$$

(Propiophenone)

Step 2: Reduction (Clemmensen or Wolff-Kishner)

$$\text{C}_6\text{H}_5\text{-CO-CH}_2\text{CH}_3 \xrightarrow{\text{Zn-Hg/HCl}} \text{C}_6\text{H}_5\text{-CH}_2\text{-CH}_2\text{CH}_3$$

Final product: n-Propylbenzene (no rearrangement!)

Answer:

  1. C₆H₆ + CH₃CH₂COCl/AlCl₃ → C₆H₅-CO-CH₂-CH₃
  2. Clemmensen reduction → C₆H₅-CH₂-CH₂-CH₃

JEE Strategy: “Can’t trust Friedel-Crafts alkylation with 1° halides? Go via acylation!”

Related: Alkanes for reduction mechanisms


Quick Revision Table

ReactionReagentElectrophileProduct
HalogenationCl₂/FeCl₃ or Br₂/FeBr₃Cl⁺ or Br⁺C₆H₅-X
NitrationHNO₃/H₂SO₄NO₂⁺C₆H₅-NO₂
SulfonationH₂SO₄ (fuming)SO₃ or HSO₃⁺C₆H₅-SO₃H
F-C AlkylationR-Cl/AlCl₃R⁺C₆H₅-R (+ rearrangement risk)
F-C AcylationRCOCl/AlCl₃RC≡O⁺C₆H₅-CO-R (no rearrangement)

Aromaticity Criteria:

  1. Cyclic ✓
  2. Planar ✓
  3. Conjugated ✓
  4. (4n+2) π electrons ✓

Connection to Other Topics

Prerequisites:

Next Topics:

Applications:


Teacher’s Summary

Key Takeaways

1. Benzene (C₆H₆) is the archetypal aromatic compound

Structure:

  • Hexagonal planar ring
  • All C-C bonds equivalent (139 pm, bond order 1.5)
  • 6 π electrons delocalized over ring
  • Resonance energy: 152 kJ/mol

2. Aromaticity Criteria (Hückel’s Rule):

Must have ALL four:

  • ✓ Cyclic structure
  • ✓ Planar geometry
  • ✓ Complete conjugation (continuous p-orbitals)
  • ✓ (4n+2) π electrons where n = 0, 1, 2, 3…

Common aromatic number: 6 π electrons (n=1)

3. Characteristic Reaction: Electrophilic Aromatic Substitution

Why substitution, not addition?

  • Substitution preserves aromaticity (retains 152 kJ/mol stability)
  • Addition destroys aromaticity (permanent loss)

General mechanism:

  1. Electrophile attacks → Arenium ion (loses aromaticity temporarily)
  2. Lose H⁺ → Restore aromaticity (fast)

4. Five Important Reactions:

ReactionKey ReagentProductRemember
HalogenationX₂/FeX₃C₆H₅-XNeed catalyst (vs alkenes)
NitrationHNO₃/H₂SO₄C₆H₅-NO₂NO₂⁺ is electrophile
SulfonationFuming H₂SO₄C₆H₅-SO₃HReversible!
F-C AlkylationRCl/AlCl₃C₆H₅-RRearrangement risk, polysubstitution
F-C AcylationRCOCl/AlCl₃C₆H₅-CO-RNo rearrangement, clean

5. JEE Strategy Points:

Aromaticity questions:

  • Always check all four criteria
  • Count π electrons carefully (4n+2 = aromatic, 4n = anti-aromatic if planar)

Mechanism questions:

  • Benzene needs stronger electrophiles (Cl⁺ not Cl₂)
  • Arenium intermediate is key
  • Deprotonation restores aromaticity

Synthesis questions:

  • Avoid F-C alkylation with 1° halides (rearrangement!)
  • Better: F-C acylation → reduction
  • Sulfonation useful for blocking positions

6. Common JEE Traps:

  • Forgetting catalyst in halogenation (benzene ≠ alkenes!)
  • Expecting addition products (benzene → substitution!)
  • Counting π bonds instead of π electrons for Hückel’s rule
  • Ignoring carbocation rearrangements in F-C alkylation

“Benzene’s aromatic stability is worth 152 kJ/mol - it will fight to keep it!”

The concept of aromaticity extends far beyond benzene - it’s the foundation for understanding all aromatic chemistry. Master these principles, and you’ll excel in aromatic compound questions!

Next, study directive effects to learn how substituents control orientation in disubstituted benzenes!